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Production of hydrogen-rich syngas and multiwalled carbon nanotubes by biogas decomposition over zirconia supported iron catalysts

Author
Pudukudy M.,Yaakob Z.,Mhd Syahri K.,Jia Q.,Shan S.
Journal Title
Journal of Industrial and Engineering Chemistry
Publication Year
2020
Topics
Summary

Fe/ZrO2 catalysts were synthesized via a urea-assisted solid-state combustion method and utilized for the thermal decomposition of undiluted biogas to produce hydrogen-rich syngas and multiwalled carbon nanotubes (MWCNTs). The catalytic activity evaluation demonstrated significantly increased methane and carbon dioxide conversion with increasing iron content and reaction temperature, achieving a maximum methane conversion of 92% and carbon dioxide conversion of 89% with an H2/CO ratio of approximately 2.25 at 900°C using the 50%Fe/ZrO2 catalyst.

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